Non-Markovian multiphoton chiral dynamics with giant systems
Yue Chang · Communications Physics · 2025
Chiral interactions enable directional control of quantum light, providing new routes for nonreciprocal photon dynamics. While previous studies focused on single photon regimes, this work explores the non-Markovian multiphoton regime in a giant nonlinear system nonlocally coupled to a one-dimensional waveguide, with a tunable phase difference breaking parity symmetry. We show that single-photon transport remains reciprocal, but multiphoton dynamics become chiral, generating direction-dependent higher-order correlations and enabling deterministic creation of multiphoton states with nontrivial statistics from a single input direction, even under strong dissipation. The non-Markovian nature allows tuning of transmitted photon statistics via the coupling-point separation. At a specific phase, internal dynamics become Markovian while output photons retain non-Markovian features. Under strong coherent driving, we uncover nonreciprocal dissipative phase transitions and demonstrate how non-Markovianity shapes the critical response. This framework offers a general strategy for controlling chiral multiphoton dynamics in nonlocally coupled waveguide QED systems. Chiral light-matter interactions offer directional control of quantum states. This work demonstrates that a giant quantum emitter with tunable nonlocal coupling to a waveguide enables direction-dependent multiphoton correlations and dissipative phase transitions, providing a route to engineer non-Markovian chiral dynamics.