Detection of photon statistics and multimode field correlations by Raman processes
Frank Schlawin, Konstantin E. Dorfman, Shaul Mukamel · The Journal of Chemical Physics · 2021
Glauber’s g(2)-function provides a common measure of quantum field statistics through two-photon coincidence counting in Hanbury Brown–Twiss measurements. Here, we propose to use nonlinear optical signals as a tool for the characterization of quantum light. In particular, we show that Raman measurements provide an alternative direct probe for a different component of the four-point correlation function underlying the g(2)-function. We illustrate this capacity for a specific quantum state obtained from a frequency conversion process. Our work points out how the analysis of controlled optical nonlinear processes can provide an alternative window toward the analysis of quantum light sources.